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* Mai Kujaku/Valentine in ''[[Yu-Gi-Oh!]]'' to Shizuka/Serenity and, to a lesser extent, Tea/Anzu.
* Urd of ''[[Ah! My Goddess]]'', to both younger sister Skuld and Keiichi on occasion, though with mixed success. Skuld seems to regard Belldandy more as her [[Cool Big Sis]] than Urd.
* Nice Holystone and eventually {{spoiler|Ennis}} from ''[[Baccano!]]''.
* Shigure Asa of ''[[
* Reki in ''[[Haibane Renmei]]'' is this to all the younger characters.
* Seiji's big sister Rin in ''[[Midori no Hibi]]'' is a mild exaggeration and subversion. Seiji's already pretty damned cool himself, but his sister is over the top -- although she dresses like an [[Office Lady]], she leads a biker gang, and generally takes all the usual Cool Big Sis behaviors to an obnoxious extreme. She's the only human being (he describes her as a demon) that he fears. She does, however, sincerely care for her little brother and wants him to be happy. Which explains why she put him through [[Training From Hell]] as a child. Of course, she ''did'' seem to enjoy it...
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